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I can't tell you how to move the iTunes root directory in Windows (probably something involving the registry), but if you just want to move all your media (music, movies, etc) to another drive you can do that from within iTunes.
In iTunes Preferences > Advanced you can select the media folder location. Pick some folder on the other hard drive and click Ok. Then, under File > Library > Organize Library consolidate or reorganise the media files. This will copy or move the files to the new location.
Cheers
Steffen.
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