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Absolutely you can, provided you can find some autoguide software that is happy to run the LPI from.
I initially trained PEC on my mount using the autoguider OTA -> Meade DSI -> ASCOM -> PHD -> Shoestring adapter -> Mount hand controller
Next step for me is to better polar align my mount and then and only then train PEC from the primary OTA not the autoguider OTA.
The next step beyond this is to do multiple training runs - throw the data into software like PEMPro to statistically average it and take the resultant master curve and upload this to your mount. Doing this would even out corrections triggered by seeing rather than mechanical properties of your mount.
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